论文标题
透射电子显微镜束中库仑相关的电子数状态
Coulomb-correlated electron number states in a transmission electron microscope beam
论文作者
论文摘要
我们证明了与飞秒光发射从透射电子显微镜内部的纳米级发射器发射的飞秒光发射的库仑相关对,三重和四倍的态。基于事件的电子光谱允许每个激光脉冲发出的电子集合的空间和光谱表征。我们确定了由加速增强的粒子室内能量交换引起的独特能量和动量相关性,揭示了大约两个电子伏特的能量尺度上的强大库仑相互作用。状态分级的梁苛性剂显示,与横向动量相关性相关的几个电子状态的虚拟源大小和纵向源移动的分散增加。我们观察到可控制的电子抗挑战,主要归因于横向库仑偏转。这些电子数态的明显空间和光谱特性允许过滤方案控制脉冲电荷的统计分布。以这种方式,可以主动抑制或增强特定的少数电子状态的比例,从而促进制备高度非磷酸电子束进行显微镜和光刻学的制备,包括未来的先驱方案和相关的多电子探测。
We demonstrate the generation of Coulomb-correlated pair, triple and quadruple states of free electrons by femtosecond photoemission from a nanoscale field emitter inside a transmission electron microscope. Event-based electron spectroscopy allows a spatial and spectral characterization of the electron ensemble emitted by each laser pulse. We identify distinctive energy and momentum correlations arising from acceleration-enhanced interparticle energy exchange, revealing strong few-body Coulomb interactions at an energy scale of about two electronvolts. State-sorted beam caustics show a discrete increase in virtual source size and longitudinal source shift for few-electron states, associated with transverse momentum correlations. We observe field-controllable electron antibunching, attributed primarily to transverse Coulomb deflection. The pronounced spatial and spectral characteristics of these electron number states allow filtering schemes that control the statistical distribution of the pulse charge. In this way, the fraction of specific few-electron states can be actively suppressed or enhanced, facilitating the preparation of highly non-Poissonian electron beams for microscopy and lithography, including future heralding schemes and correlated multi-electron probing.