论文标题
无序晶体揭示了柔软的准化玻璃兴奋
Disordered crystals reveal soft quasilocalized glassy excitations
论文作者
论文摘要
众所周知,通过淬灭融化而形成的结构玻璃可以容纳低能量的准定位(非传播)激发,其频率$ω$遵循通用的$ \ sim \ sim \!ω^4 $分布为$ω\!\!在这里,我们表明,非传声激发的通用四分之一定律也具有有限的远距离顺序的无序晶体,其玻璃型同行中不存在。因此,我们确定四分之一定律的普遍性超出了从熔体中消失的结构眼镜。我们进一步发现,与基于机械障碍的程度相比,与剪切模量的相对波动量化的无序晶体可以连续控制其疾病水平,与预期的相比,与具有类似机械障碍程度的结构玻璃相比,其量化激发比预期的。最后,我们表明,稳定性结合在非线性准定位激发(以前以结构玻璃为基础)中建立的稳定性也具有无序的晶体。我们的结果与在无序晶体中实验观察到的玻璃样异常有关。更广泛地说,它们构成了追踪无序固体中普遍非传声激发所必需的基本要素迈出的重要一步。
Structural glasses formed by quenching a melt are known to host a population of low-energy quasilocalized (nonphononic) excitations whose frequencies $ω$ follow a universal $\sim\!ω^4$ distribution as $ω\!\to\!0$, independently of the glass formation history, the interparticle interaction potential or spatial dimension. Here, we show that the universal quartic law of nonphononic excitations also holds in disordered crystals featuring finite long-range order, which is absent in their glassy counterparts. We thus establish that the degree of universality of the quartic law extends beyond structural glasses quenched from a melt. We further find that disordered crystals, whose level of disorder can be continuously controlled, host many more quasilocalized excitations than expected based on their degree of mechanical disorder -- quantified by the relative fluctuations of the shear modulus -- as compared to structural glasses featuring a similar degree of mechanical disorder. Finally, we show that the stability bound on nonlinear quasilocalized excitations -- previously established in structural glasses -- also holds in disordered crystals. Our results are related to glass-like anomalies experimentally observed in disordered crystals. More broadly, they constitute an important step towards tracing the essential ingredients necessary for the emergence of universal nonphononic excitations in disordered solids.