论文标题
在中等磁场下,自旋冰材料中的异常异常动力学$ _2 $ _2 $ _2 $ o $ _7 $
Anomalous out-of-equilibrium dynamics in the spin-ice material Dy$_2$Ti$_2$O$_7$ under moderate magnetic fields
论文作者
论文摘要
我们通过实验和数字研究自旋冰材料的动态$ _2 $ _2 $ _2 $ o $ $ _7 $在低温($ t $)和中等磁场($ \ m m i \ mathbf {b} $)方案($ t \ in [0.1,1.7] k $,$ b \ in [0.1.7] k $ in [0.1.7] k $ in [0,0,0.3] t $)t $)。我们的目标是了解在两个不同的方案中塑造过平衡磁化与温度曲线的主要物理学。离平衡很远,在零场(ZFC)冷却系统后打开磁场可以增加磁性单极的浓度。这加速了动态。与电解质类似,这是通过结合单极对的解离。但是,对于自旋冰而言,创建单极对的真空极化是塑造磁化曲线的关键因素,而没有类似物。我们观察到一个接近$ 0.2T $的门槛场,以供此快速动态进行,与吸引对之间的最大磁力有关。令人惊讶的是,在低温和中等场的制度中,可以使用扩展的欧姆定律来描述用偶极旋转冰模型获得的ZFC磁化曲线。但是,在实际样品中,动态的加速度似乎比模拟更明显,这可能是由于存在雪崩所致。另一方面,在非常低的温度下,较接近平衡的田间效果可能相反。如前所述,单晶在阻塞温度下放弃了平衡,随着场的增加。奇怪的是,即使在最近的近港相互作用模型中,这种行为也存在于数值模拟中。仿真和实验表明,$ t_b $的趋势增加的趋势对于$ \ mathbf {b} \ Parallel [100] $都更强。这表明该领域通过单极抑制在动态停滞中起着作用,这在该领域方向很明显。
We study experimentally and numerically the dynamics of the spin ice material Dy$_2$Ti$_2$O$_7$ in the low temperature ($T$) and moderate magnetic field ($\mathbf{B}$) regime ($T\in[0.1,1.7]K$, $B\in[0,0.3]T$). Our objective is to understand the main physics shaping the out-of-equilibrium magnetisation vs. temperature curves in two different regimes. Very far from equilibrium, turning on the magnetic field after having cooled the system in zero field (ZFC) can increase the concentration of magnetic monopoles; this accelerates the dynamics. Similarly to electrolytes, this occurs through dissociation of bound monopole pairs. However, for spin ices the polarisation of the vacuum out of which the monopole pairs are created is a key factor shaping the magnetisation curves, with no analog. We observe a threshold field near $0.2T$ for this fast dynamics to take place, linked to the maximum magnetic force between the attracting pairs. Surprisingly, within a regime of low temperatures and moderate fields, an extended Ohm's law can be used to describe the ZFC magnetisation curve obtained with the dipolar spin-ice model. However, in real samples the acceleration of the dynamics appears even sharper than in simulations, possibly due to the presence of avalanches. On the other hand, the effect of the field nearer equilibrium can be just the opposite to that at very low temperatures. Single crystals, as noted before for powders, abandon equilibrium at a blocking temperature $T_B$ which increases with field. Curiously, this behaviour is present in numerical simulations even within the nearest-neighbours interactions model. Simulations and experiments show that the increasing trend in $T_B$ is stronger for $\mathbf{B}\parallel[100]$. This suggests that the field plays a part in the dynamical arrest through monopole suppression, which is quite manifest for this field orientation.